By Author Unknown, William L Hase
This moment quantity within the sequence covers such themes as lengthy lived ion complexes, crossed beam experiences on ion-moleculaar reactions, the double-well version for ion-molecule reactions and intricate formation, and direct collision dynamics in fuel section nucleophilic substitution reactions
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The solid line is drawn through the points. The rates are drawn from data of Werner and Baer. absorbed by the butadiene ions, which results in the production of C3H3+ ions. On the other hand, the butyne ions cannot absorb the visible laser light. However, as the butyne ion internal energy is increased, it reaches an internal energy at which it can isomerize to the butadiene structure, whereupon it absorbs the laser light. Thus, the onset of C3H3+ product signals the onset of isomerization to the lower energy butadiene ion structure.
1980, 99. 24. Truhlar, D. ; Garrett, B. C. Ace. Chem. Res. 1980,13, 440. 25. Chesnavich, W. ; Bowers, M. T. J. Chem. Phys. 1981, 74, 2228. 26. ; Troe, J. Ber. Bunsenges. Physik. Chem. 1973, 77, 24. 27. ; Troe, J. Ber. Bunsenges. Physik. Chem. 1974, 78, 240. 28. Marcus, R. ; Rice, O. K. J. Phys. Colloid Chem. 1951, 55, 894. 29. Rosenstock, H. ; Wallenstein, M. ; Wahrhaftig, A. ; Eyring, H. Proc. Nati. Acad. Sci. USA 1952, 38, 667. 30. ; Weitzel, K. M. In Vacuum Ultraviolet lonization and Dissociation of Molecules and Clusters; C.
Despite the breadth of this distribution, it is clear that the HCO+ products formed from this process are fairly "hot" internally. 7 eV corresponds to over 50% of the available energy. The kinetic energy distribution, from which one can infer the internal energy distribution in the HCO+ product, is quite broad but suggests that the products are significantly "colder" internally than those produced at the higher collision energy. These kinetic energy distributions provide some important constraints on product identity.